Not relaxed

The answer to this crossword clue is “Edgy.” The word “Edgy” means being in a state of nervous tension or agitation, which is the polar opposite of being relaxed. If someone is described as not relaxed, it implies that they are tense or anxious, which is synonymous with being edgy. Additionally, the word “Edgy” can also be used to mean being sharp or having a pointed edge, but in this context, it refers to a person’s emotional state. Therefore, the answer to this clue is “Edgy.”